Volume 37 Issue 1
Mar.  2023
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YAN Jinbiao, WANG Sha, ZHANG Huarong. Research progress of carbon deposition resistance of catalyst for dry reforming of methane to hydrogen[J]. Journal of Shanghai University of Engineering Science, 2023, 37(1): 1-6, 40. doi: 10.12299/jsues.22-0093
Citation: YAN Jinbiao, WANG Sha, ZHANG Huarong. Research progress of carbon deposition resistance of catalyst for dry reforming of methane to hydrogen[J]. Journal of Shanghai University of Engineering Science, 2023, 37(1): 1-6, 40. doi: 10.12299/jsues.22-0093

Research progress of carbon deposition resistance of catalyst for dry reforming of methane to hydrogen

doi: 10.12299/jsues.22-0093
  • Received Date: 2022-04-21
  • Publish Date: 2023-03-31
  • Among modern industrial hydrogen production technologies, methane reforming for hydrogen production has unique advantages in rich reactant sources and high availability, especially dry reforming of methane (DRM) technology, which uses methane and carbon dioxide as raw materials and has both environmental and economic benefits. Carbon deposition on catalyst is one of the main problems affecting the development of DRM technology. To design high-performance catalysts, current research mainly focuses on the active components, supports, and promoters. This article discusses in detail the effects of interaction between active components and supports, active metal particle size, basicity, oxygen storage capacity, and carbon deposition type on the carbon deposition resistance of DRM catalysts. The results indicate that strong interactions between active metals and supports, synergistic effects of bimetallic catalysts, and smaller active metal particles can reduce carbon deposition and improve catalyst activity. Increasing oxygen storage capacity can promote carbon removal. The type and amount of carbon deposition are closely related to the support material, and moderate support basicity can promote CO2 activation, thereby improving the carbon deposition resistance of the catalyst. This article provides a reference for the design and optimization of DRM catalysts.
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