Volume 37 Issue 2
Jun.  2023
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ZOU Jingtao, LI Xuankun, YANG Jie, WEI Mingfei, ZHANG Wenqi, LI Guanghui. Preparation of photocatalytic ozonation SiC foam and its application in levofloxacin degradation[J]. Journal of Shanghai University of Engineering Science, 2023, 37(2): 113-119. doi: 10.12299/jsues.22-0189
Citation: ZOU Jingtao, LI Xuankun, YANG Jie, WEI Mingfei, ZHANG Wenqi, LI Guanghui. Preparation of photocatalytic ozonation SiC foam and its application in levofloxacin degradation[J]. Journal of Shanghai University of Engineering Science, 2023, 37(2): 113-119. doi: 10.12299/jsues.22-0189

Preparation of photocatalytic ozonation SiC foam and its application in levofloxacin degradation

doi: 10.12299/jsues.22-0189
  • Received Date: 2022-06-21
  • Publish Date: 2023-06-20
  • To solve the problem of environmental pollution caused by the difficult degradation of antibiotics, Ce-TiO2/SiC foam was prepared, levofloxacin (Levofloxacin, LEV) was chosen as the target pollutant, and a photocatalytic ozonation coupling system (Ce-TiO2/SiC + LED + O3) was studied. The results show that the coupling system can effectively degrade LEV, the LEV removal was 99% and the chemical oxygen demand (COD) removal was as high as 85.9%. The coupling system showed a good synergistic effect, and its first-order reaction kinetic rate constant was greater than the sum of ozonation (O3) and photocatalysis (Ce-TiO2/SiC + LED). In addition, the stability experiment of Ce-TiO2/SiC foam showed that the photocatalytic ozonation activity is basically unchanged after five reuses.
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  • [1]
    张万鹏, 郑立庆, 杨鑫雨, 等. 球磨−煅烧法制备Fe3O4-CuxO及其活化Oxone降解盐酸左氧氟沙星[J] . 中国环境科学,2020,40(1):143 − 152. doi: 10.3969/j.issn.1000-6923.2020.01.016
    [2]
    LYU J, YANG L S, ZHANG L, et al. Antibiotics in soil and water in China: A systematic review and source analysis[J] . Environmental Pollution,2020,266:115147. doi: 10.1016/j.envpol.2020.115147
    [3]
    LI Z, LI M, ZHANG Z Y, et al. Antibiotics in aquatic environments of China: A review and meta-analysis[J] . Ecotoxicology and Environmental Safety,2020,199:110668.
    [4]
    XIA Y J, DAI Q Z. Electrochemical degradation of antibiotic levofloxacin by PbO2 electrode: Kinetics, energy demands and reaction pathways[J] . Chemosphere,2018,205:215 − 222. doi: 10.1016/j.chemosphere.2018.04.103
    [5]
    JOSHI S M, GOGATE P R. Treatment of landfill leachate using different configurations of ultrasonic reactors combined with advanced oxidation processes[J] . Separation and Purification Technology,2019,211:10 − 18. doi: 10.1016/j.seppur.2018.09.060
    [6]
    朱晓兵, 金灿, 李小松, 等. LED可见光下Au/TiO2光催化氧化甲醛表观动力学[J] . 化工学报,2017,68(S1):196 − 203.
    [7]
    BUYUKADA M. Removal, potential reaction pathways, and overall cost analysis of various pollution parameters and toxic odor compounds from the effluents of turkey processing plant using TiO2 assisted UV/O3 process[J] . Journal of Environmental Management,2019,248:109298. doi: 10.1016/j.jenvman.2019.109298
    [8]
    LI Y H, CHENG S W, YUAN C S, et al. Removing volatile organic compounds in cooking fume by nano-sized TiO2 photocatalytic reaction combined with ozone oxidation technique[J] . Chemosphere,2018,208:808 − 817. doi: 10.1016/j.chemosphere.2018.06.035
    [9]
    XIE Y B, YANG J, CHEN Y, et al. Promising application of SiC without co-catalyst in photocatalysis and ozone integrated process for aqueous organics degradation[J] . Catalysis Today,2018,315:223 − 229. doi: 10.1016/j.cattod.2018.01.013
    [10]
    SUZUKI H, ARAKI S, YAMAMOTO H. Evaluation of advanced oxidation processes (AOP) using O3, UV, and TiO2 for the degradation of phenol in water[J] . Journal of Water Process Engineering,2015,7:54 − 60. doi: 10.1016/j.jwpe.2015.04.011
    [11]
    ZHU Q Y, WANG Y Q, WANG L X, et al. Solvent-free crystallization of ZSM-5 zeolite on SiC foam as a monolith catalyst for biofuel upgrading[J] . Chinese Journal of Catalysis,2020,41(7):1118 − 1124. doi: 10.1016/S1872-2067(20)63550-1
    [12]
    M'BRA I C, GARCÍA-MUÑOZ P, DROGUI P, et al. Heterogeneous photodegradation of Pyrimethanil and its commercial formulation with TiO2 immobilized on SiC foams[J] . Journal of Photochemistry & Photobiology A:Chemistry,2019,368:1 − 6.
    [13]
    WANG Y P, KE L Y, PENG Y J, et al. Ex-situ catalytic fast pyrolysis of soapstock for aromatic oil over microwavedriven HZSM-5@SiC ceramic foam[J] . Chemical Engineering Journal,2020,402:126239. doi: 10.1016/j.cej.2020.126239
    [14]
    TOUATI A, HAMMEDI T, NAJJARA W, et al. Photocatalytic degradation of textile wastewater in presence of hydrogen peroxide: Effect of cerium doping titania[J] . Journal of Industrial and Engineering Chemistry,2016,35:36 − 44. doi: 10.1016/j.jiec.2015.12.008
    [15]
    KONSTANTINOU I K, ALBANIS T A. TiO2-assisted photocatalytic degradation of azo dyes in aqueous solution: kinetic and mechanistic investigations: A review[J] . Applied Catalysis B: Environmental,2004,49(1):1 − 14. doi: 10.1016/j.apcatb.2003.11.010
    [16]
    LING Y, LIAO G Z, XIE Y H, et al. Coupling photocatalysis with ozonation for enhanced degradation of atenolol by Ag-TiO2 micro-tube[J] . Journal of Photochemistry and Photobiology A: Chemistry,2016,329:280 − 286. doi: 10.1016/j.jphotochem.2016.07.007
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